CPOTE2026
|
9th
International Conference on
Contemporary Problems of Thermal Engineering
23-25 September 2026 | Kraków, Poland | In-person
Contemporary Problems of Thermal Engineering
23-25 September 2026 | Kraków, Poland | In-person
Abstract CPOTE2026-6026-A
CUPOLA: Beyond barriers - collaborative approaches to carbon-neutral recycling of marine plastic waste
Aneta MAGDZIARZ, AGH University of Kraków, PolandZheng WANG, University of Nottingham Ningbo China, China
Agata MLONKA-MĘDRALA, AGH University of Krakow, Poland
Chunfei WU, Queen’s University Belfast, United Kingdom of Great Britain and Northern Ireland
Marcin SAJDAK, Silesian University of Technology, Poland
Gillian COLLINS, University College Cork, Ireland
James A. SULLIVAN, University College Dublin, Ireland
Jiawei WANG, Swansea University, United Kingdom of Great Britain and Northern Ireland
Marine plastic waste (MPW) is a complex and contaminated waste stream that poses significant challenges for recycling with traditional methods. The CUPOLA project aims to address this issue by developing integrated, carbon-neutral processes for sorting and converting MPW into valuable chemicals, carbon materials, and functional products. This initiative involves separating MPW into PET-rich, polyolefin-rich, and polyamide-rich fractions, followed by customised recycling and upgrading pathways, all supported by process modelling and environmental assessments.
The conversion of PET-rich municipal plastic waste can produce high-value intermediates for road applications. Glycolysis enables the recovery of terephthalic acid in high purity, whereas aminolysis yields terephthalamide-based compounds with reactive hydroxyl and amide functionalities, making them suitable for bitumen modification. Furthermore, the reported results indicate that the glycolysis route has a favourable environmental performance, highlighting its potential as a sustainable method for PET valorisation. The catalytic conversion of polyolefin-rich MPW, showed strong potential for producing BTX aromatics, hydrogen, and carbon nanotubes. Ex-situ catalytic pyrolysis achieved conversion efficiencies above 98 wt. %, with aromatic compounds dominating the liquid fraction, while catalytic vapour deposition routes enabled the simultaneous generation of hydrogen and carbon nanomaterials. Additionally, MPW-derived products can serve as functional carbon materials and CO2 capture media. The PA-rich MPWs were valorised for fibre regeneration and the production of nitrogen-rich carbonaceous materials.
Beyond the technical results, CUPOLA is fundamentally a collaboration- and knowledge-transfer-driven project. It was designed as an international, interdisciplinary and intersectoral programme connecting universities across Europe and Asia to develop long-term research cooperation in marine plastic waste recycling. A core project objective is the transfer of knowledge through staff exchanges, training schools, workshops, enabling mutual learning across disciplines such as waste sorting, chemical recycling, process modelling, life cycle assessment, and techno-economic analysis. In this sense, CUPOLA is not only developing new valorisation routes for MPW, but also building the research capacity, shared expertise, and collaborative framework needed for their future implementation.
Keywords: Marine plastic waste, CO2, Pyrolysis, Gasification, Carbon materials
Acknowledgment: This project has received funding from the European Union HORIZON TMA MSCA Staff Exchanges (HORIZON-MSCA-2021-SE-01), grant agreement no 101086071, project name “CUPOLA — Carbon-neutral pathways of recycling marine plastic waste”. Support was also provided by the Ministry of Science and Higher Education in Poland through the program "PMW grant no. 5863/HE/2024/2 (no. W52/HE/2024).